Optically Active Charge Traps and Chemical Defects in Semiconducting Nanocrystals Probed by Pulsed Optically Detected Magnetic Resonance
(Sprache: Englisch)
This book lays the groundwork for further use of Electron Spin Echo Envelop Modulation (ESEEM) and opens the possibility of highly precise chemical fingerprinting. It reveals an astonishingly long memory of spin coherence in semiconductor particles.
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This book lays the groundwork for further use of Electron Spin Echo Envelop Modulation (ESEEM) and opens the possibility of highly precise chemical fingerprinting. It reveals an astonishingly long memory of spin coherence in semiconductor particles.
Klappentext zu „Optically Active Charge Traps and Chemical Defects in Semiconducting Nanocrystals Probed by Pulsed Optically Detected Magnetic Resonance “
Colloidal nanocrystals show much promise as an optoelectronics architecture due to facile control over electronic properties afforded by chemical control of size, shape, and heterostructure. Unfortunately, realizing practical devices has been forestalled by the ubiquitous presence of charge "trap" states which compete with band-edge excitons and result in limited device efficiencies. Little is known about the defining characteristics of these traps, making engineered strategies for their removal difficult.This thesis outlines pulsed optically detected magnetic resonance as a powerful spectroscopy of the chemical and electronic nature of these deleterious states. Counterintuitive for such heavy atom materials, some trap species possess very long spin coherence lifetimes (up to 1.6 µs). This quality allows use of the trapped charge's magnetic moment as a local probe of the trap state itself and its local environment. Beyond state characterization, this spectroscopy can demonstrate novel effects in heterostructured nanocrystals, such as spatially-remote readout of spin information and the coherent control of light harvesting yield.
Inhaltsverzeichnis zu „Optically Active Charge Traps and Chemical Defects in Semiconducting Nanocrystals Probed by Pulsed Optically Detected Magnetic Resonance “
Introduction.- Experimental Methods.- Spin-Dependent Exciton Quenching and Intrinsic Spin Coherence in CDSE/CDS Nanocrystals.- Towards Chemical Fingerprinting of Deep-Level Defect Sites in CDS Nanocrystals by Optically Detected Spin Coherence.- Summary of Work.
Autoren-Porträt von Kipp van Schooten
Kipp van Schooten Department of Physics and Astronomy
University of Utah
Salt Lake City, UT, 84112
USA
Kipp van Schooten received his Ph.D. in Physics (Condensed Matter focus) from the University of Utah in December 2012. He received the Outstanding Teaching Assistant award each year from 2005 - 2009 for the courses "Intro to Quantum Relativity" and "Solid State Physics II." In 2011, he also received first place for Best Graduate Student Oral Presentation at the University of Utah.
Bibliographische Angaben
- Autor: Kipp van Schooten
- 2015, Softcover reprint of the original 1st ed. 2013, XIV, 90 Seiten, 90 farbige Abbildungen, Maße: 15,5 x 23,5 cm, Kartoniert (TB), Englisch
- Verlag: Springer, Berlin
- ISBN-10: 331903328X
- ISBN-13: 9783319033280
Sprache:
Englisch
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